한빛사논문
Kiyoung Jo1, Emanuele Marino2,3, Jason Lynch1, Zhiqiao Jiang2,4, Natalie Gogotsi4, Thomas P. Darlington5, Mohammad Soroush6, P. James Schuck5, Nicholas J. Borys6, Christopher B. Murray2,4 & Deep Jariwala1
1Department of Electrical and Systems Engineering, University of Pennsylvania, Philadelphia, PA 19104, USA.
2Department of Chemistry, University of Pennsylvania, Philadelphia, PA 19104, USA.
3Dipartimento di Fisica e Chimica, Università degli Studi di Palermo, Via Archirafi 36, 90123 Palermo, Italy.
4Department of Materials Science and Engineering, University of Pennsylvania, Philadelphia, PA 19104, USA.
5Department of Mechanical Engineering, Columbia University, New York, NY 10027, USA.
6Departement of Physics, Montana State University, Bozeman, MT 59717, USA.
Corresponding author : Correspondence to Deep Jariwala.
Abstract
Strong light-matter interactions in localized nano-emitters placed near metallic mirrors have been widely reported via spectroscopic studies in the optical far-field. Here, we report a near-field nano-spectroscopic study of localized nanoscale emitters on a flat Au substrate. Using quasi 2-dimensional CdSe/CdxZn1-xS nanoplatelets, we observe directional propagation on the Au substrate of surface plasmon polaritons launched from the excitons of the nanoplatelets as wave-like fringe patterns in the near-field photoluminescence maps. These fringe patterns were confirmed via extensive electromagnetic wave simulations to be standing-waves formed between the tip and the edge-up assembled nano-emitters on the substrate plane. We further report that both light confinement and in-plane emission can be engineered by tuning the surrounding dielectric environment of the nanoplatelets. Our results lead to renewed understanding of in-plane, near-field electromagnetic signal transduction from the localized nano-emitters with profound implications in nano and quantum photonics as well as resonant optoelectronics.
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